Title

Direct conversion of methane to higher hydrocarbons using AlBr3-HBr superacid catalyst

Document Type

Article

Publication Date

1-14-2011

Abstract

The direct gas phase catalytic oligomerization of methane at temperatures ≤673 K has been demonstrated using AlBr(3)-HBr superacid. The reaction produces C(2)+ hydrocarbons and hydrogen in a single step at 1 atm in a continuous flow reactor at a nominal residence time of 60 s. The essentially complete conversion of methane appears to be due to protolytic activation of methane in the presence of H(+)AlBr(4)(-).

Publication Source (Journal or Book title)

Chemical communications (Cambridge, England)

First Page

785

Last Page

7

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