We investigate the evolution of extreme ultraviolet (XUV) spectral line shapes in an optically thick helium gas under near-infrared (IR) perturbation. In our experimental and theoretical work, we systematically vary the IR intensity, time-delay, gas density, and IR polarization parameters to study line-shape modifications induced by collective interactions in a regime beyond the single-atom response of a thin, dilute gas. In both experiment and theory, we find that specific features in the frequency-domain absorption profile, and their evolution with propagation distance, can be attributed to the interplay between resonant attosecond pulse propagation and IR-induced phase shifts. Our calculations show that this interplay also manifests itself in the time domain, with the IR pulse influencing the reshaping of the XUV pulse propagating in the resonant medium.
Publication Source (Journal or Book title)
Physical Review A
Liao, C., Sandhu, A., Camp, S., Schafer, K., & Gaarde, M. (2016). Attosecond transient absorption in dense gases: Exploring the interplay between resonant pulse propagation and laser-induced line-shape control. Physical Review A, 93 (3) https://doi.org/10.1103/PhysRevA.93.033405