Comparison of the use of different solubility models for the cooling crystallization of acetaminophen

Document Type

Conference Proceeding

Publication Date

12-1-2008

Abstract

In this paper we evaluate the sensitivity of using different solubility models on the cooling crystallization of acetaminophen. Empirical, correlative thermodynamic (namely NRTL) and predictive thermodynamic (namely MOSCED) models are considered. Equilibrium solubility model prediction determines the predicted supersaturation profile. The different solubility equations are used within a population balance model for prediction of crystal size properties. Incorrect prediction of the supersaturation profile results in incorrect prediction of crystal size distribution. The NRTL model was found to be more accurate at predicting equilibrium solubility and consequently crystal size. After the solubility sensitivity is evaluated, two methods are proposed to make the crystallization model more robust against solubility model errors.

Publication Source (Journal or Book title)

AIChE Annual Meeting, Conference Proceedings

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